Abstract:
Conventional quantum dissipation theory is often limited to model systems
which contain a few levels, while quantum chemistry methods are routinely
applied to real complex systems containing hundreds or thousands of
orbitals. Basing on the holographic electron density theorem, an exact
first-principles framework is proposed for open systems, in particular, a
time-dependent density-fucntional theory is developed for quantum transport,
and has been applied to simulate the transient currents through various
nanoscopic electronic devices. In particular, transient currents through a
set of metallic wires of different sizes are calculated, and a surprising
linear relationship between the current and time is observed.
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